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Daily Crossword Puzzle #4 for Fri, Dec 17, 2021

ACROSS
1. Nervous spasm
4. Mail
8. Is not
12. Smallest unit of an element
14. Toward the sea
15. Letter starter
16. Cause to be
17. Unrelated to defense, as in spending
20. Downhill vehicle
21. Compass dir.
22. Had dinner
23. Religious groups
27. Stricken, poetically
29. Curves
31. Be footloose
34. Bee-related
35. Roberta Peters solo
36. Soap bubbles
39. Modern: prefix
41. Russian ruler of old
42. Angers
43. Take place subsequently
46. Cause heat under the collar
47. Relief
48. Of or related to the anus
51. Bull
54. Put into a specified state
56. French article
58. Frog relative
61. The property of being fit to eat
66. Native american tent (variation)
67. Small Philippine buffalo
68. Toward shelter
69. In addition
70. Austrian-born American filmmaker Fritz
71. Entreaty
72. It is so

DOWN
1. Scottish caps
2. Slanted text style (abbr.)
3. Popular sodas
4. Baking dish
5. Bear (Spanish)
6. Elected rep.
7. Bits
8. Binary compound
9. Legislators
10. Political cartoonist Thomas
11. Woody plant
13. Ancient Persian
18. Curvy letter
19. Opposite of masc.
24. Head covering
25. Three (prefix)
26. Examine minutely or intensely
28. Feeling or showing extreme anger
30. Contemptuous expression
32. By way of
33. Ewer handle
34. NE Netherlands city
36. Title for a knight
37. RI univ.
38. Accusation by an informer
40. Washington bills
44. Fast jet (abbr.)
45. Shoshoni
49. Everything
50. Area sheltered from the wind
52. Singer James
53. Agitated, as a liquid
54. Lick closed
55. Pulitzer Prize-winning author Ferber
57. Fastener
59. Domed church section
60. "Vaya con ____"
62. Paper or plastic container
63. Pipe bend
64. Observe
65. Ocean